Dynamical structure factor of the three-dimensional quantum spin liquid candidate NaCaNi2F7
霍普金斯大学 Shu "Suzy" Zhang, Johns Hopkins University
报告摘要:
To look for quantum spin liquid states in real materials, it is crucial to understand the dynamical signatures in their magnetic excitations. The spin-1 compound NaCaNi2F7[1] is an almost ideal realization of the antiferromagnetic Heisenberg model on a pyrochlore lattice, the classical version of which is predicted to be a spin liquid[2]. Indeed, the material doesn’t develop magnetic order down to 0.35K and the broad continuum observed in the inelastic neutron scattering experiment[3] indicates the absence of magnons with well-defined dispersions. We theoretically calculate the dynamical structure factor using three complementary methods: molecular dynamics, stochastic model and the linear spin wave theory. The results[4] reproduce well the momentum and energy dependence of the scattering intensity. This analysis leads to an intuitive picture of the spin dynamics in this frustrated magnet.
[1] J. W. Krizan and R. J. Cava, Phys. Rev. B 92, 014406 (2015)
[2] S. V. Isakov, K. Gregor, R. Moessner, and S. L. Sondhi, Phys. Rev. Lett. 93, 167204 (2004)
[3] K. W. Plumb, H. J. Changlani, A. Scheie, S. Zhang, J. W. Krizan, J. A. Rodriguez- Rivera, Y. Qiu, B. Winn, R. J. Cava and C. L. Broholm, Nat. Phys. 10.1038/s41567- 018-0317-3 (2018)
[4] S. Zhang, H. J. Changlani, K. W. Plumb, O. Tchernyshyov and R. Moessner, arXiv:1810.09481
联系人:万源 yuan.wan@iphy.ac.cn